Adding on to this to specifically recommend the Castlevania: Lords of Shadow 2 soundtrack. Oscar Araujo did masterful work on this, so much so that I even went out and bought the album, even though it was almost impossible to get my hands on it. But you can listen to it on YouTube.
It’s great stuff. As a bonus, an artist named Alex Yarmak has put together two albums where he covers the entire OST of each game in a heavy metal style. Great stuff if you like that kind of thing.
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